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1、iffsSi'ALKALI-DOPEDFULLERIDESNarrow-BandSolidswithUnusualPropertiesOlleGunnarssonALKALI-DOPEDFULLERIDESNarrow-BandSolidswithUnusualPropertiesThispageisintentionallyleftblankALKALI-DOPEDFULLERIDESNarrow-BandSolidswithUnusualPropertiesOlleGunnarssonMax-Planck-Institutfu?-Festk6fpef
2、forschtmg^PWorldScientificNEWJERSEY*LONDON•SINGAPORE•BEIJING•SHANGHAI•HONGKONG•TAIPEI*CHENNAIPublishedbyWorldScientificPublishingCo.Pte.Ltd.5TohTuckLink,Singapore596224USAoffice:Suite202,1060MainStreet,RiverEdge,NJ07661UKoffice:57SheltonStreet,CoventGarden,LondonWC2H9HEBritishLib
3、raryCataloguing-in-PublicationDataAcataloguerecordforthisbookisavailablefromtheBritishLibrary.ALKALI-DOPEDFULLERIDES:NARROW-BANDSOLIDSWITHUNUSUALPROPERTEESCopyright©2004byWorldScientificPublishingCo.Pte.Ltd.Allrightsreserved.Thisbookorpartsthereof,maynotbereproducedinanyformorbya
4、nymeans,electronicormechanical,includingphotocopying,recordingoranyinformationstorageandretrievalsystemnowknownortobeinvented,withoutwrittenpermissionfromthePublisher.Forphotocopyingofmaterialinthisvolume,pleasepayacopyingfeethroughtheCopyrightClearanceCenter,Inc.,222RosewoodDriv
5、e,Danvers,MA01923,USA.Inthiscasepermissiontophotocopyisnotrequiredfromthepublisher.ISBN981-238-667-XPrintedinSingaporebyWorldScientificPrinters(S)PteLtdToLauraThispageisintentionallyleftblankPrefaceThediscoveryoffullerenes,e.g.,Cgo,byKrotoetal.1in1985createdgreatexcitement,andin1
6、996,Curl,KrotoandSmalleyreceivedtheNobelprizeinchemistryfortheirdiscovery.Initially,theinterestwasinparticularduetotheappealingsymmetricshapeoftheCQQmolecule,whichhasthehighestpossiblepointgroupsymmetry.However,researchwashamperedbytheminuteamountsoffullerenesavailable.Thiscomple
7、telychangedwhenKratschmeretal.2discoveredhowtoproduceCeoinlargequantitiesin1990.Itthenbecamepossibletoperformalargenumberofsolidstatephysicsexperiments.Verysoon,Haddonetal.3foundthatintercalationofalkalimetalatomsintosolidCeoleadstometallicbehavior.Shortlythereafter,Hebardetal.4a
8、ndseveralothergroups5'6,7'8foundthatsome